I am now going to get a rough idea of how much caesium 137 there is in spent nuclear fuel. One reason for choosing Cs-137 is that it is a major fission product, it has a reasonably long half-life (30.17 years), it has a low melting and boiling point and is readily absorbed by the human body.
I am going to assume that the Cs-137 does not decay to any appreciable amount while it is in the reactor. This is just to make this post a bit simpler, and I have shown how to take this into account in this post if anyone is interested.
I have shown how to get a rough idea of how many fission events are necessary to produce a certain amount of energy, and expressed this as fissions per tonne of Uranium in a Rough Model of a Nuclear Reactor.I have also given data on now many atoms of a particular isotope is produced per fission in Composition of Spent Fuel.
So now we can simply multiply the two numbers – i.e. number of fissions per tonne of Uranium by the probability that a certain isotope (in this case Cs-137) will be produced.
For example, if there are 1.33×1026 fissions per tonne of uranium and 6% of them result in an atom of Cs-137 then we would expect 1.33×1026 x 0.06 = 7.97 x 1024 atoms of Cs-137 to be produced. We can then compare it with published data.
Number of fission product atoms per gram of uranium | |||
Burnup GWDays/TU | Measured1 | Calculated: basic model | Calculated: advanced model |
0.00 | 0.00E+000 | 0.00E+000 | 0.00E+000 |
1.20 | 1.94E+017 | 2.04E+017 | 1.94E+017 |
4.70 | 7.63E+017 | 8.00E+017 | 7.60E+017 |
9.90 | 1.60E+018 | 1.69E+018 | 1.60E+018 |
15.10 | 2.43E+018 | 2.57E+018 | 2.44E+018 |
20.00 | 3.17E+018 | 3.41E+018 | 3.24E+018 |
25.60 | 4.05E+018 | 4.36E+018 | 4.14E+018 |
29.60 | 4.64E+018 | 5.04E+018 | 4.79E+018 |
34.70 | 5.40E+018 | 5.91E+018 | 5.61E+018 |
40.00 | 6.15E+018 | 6.81E+018 | 6.47E+018 |
46.80 | 7.14E+018 | 7.97E+018 | 7.57E+018 |
The basic model is where I have assumed that the Cs-137 does not undergo decay in the reactor whereas the more advanced model takes this decay into account.
Not bad for such a rough model. However, this is the amount of Cs-137 in the fuel as it leaves the reactor. Once out of the reactor it is no longer being produced but simply decays. I shall look at this in a later post.
1 Irradiated Fuel Measurements, J. Parker (http://www.fas.org/sgp/othergov/doe/lanl/lib-www/la-pubs/00326413.pdf)
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